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Centre de Recherches en Physique des Plasmas. Material erosion and migration in tokamaks. R. A. Pitts CRPP, Association-EURATOM Conf é d é ration Suisse, EPFL Lausanne, Switzerland. with many thanks for contributions from
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Centre de Recherches en Physique des Plasmas Material erosion and migration in tokamaks • R. A. Pitts • CRPP, Association-EURATOM Confédération Suisse, EPFL Lausanne, Switzerland • with many thanks for contributions from • N. Asakura1, S. Brezinsek2, C. Brosset3, J. P. Coad4, D. Coster5, E. Dufour3, G. Federici6, R. Felton4, M. E. Fenstermacher7, R. S. Granetz8, A. Herrmann5, J. Horacek, A. Kirschner2, K. Krieger5, A. Loarte9, J.Likonen10, B. Lipschultz8, A. Kukushkin6, G. F. Matthews4, M. Mayer5, R. Neu5, J. Pamela11, B. Pégourié3, V. Philipps2, J. Roth5, M. Rubel12, L. L. Snead13, P. C. Stangeby14, J.D. Strachan15, E. Tsitrone3, W. Wampler16, D. Whyte17 • 1JAERI, 2FZJ-Jülich, 3CEA Cadarache, 4UKAEA, 5IPP Garching, 6ITER, 7LLNL, 8PSFC-MIT, 9EFDA CSU Garching, 10VTT-TEKES, 11EFDA CSU Culham, 12Alfvén Lab. RIT, 13ORNL, 14UTIAS, 15PPPL, 16SNL,17Univ. Wisconsin,
Outline of the talk • Introduction • The components of migration • Global migration accounting • Material choices for the next step • Conclusions
What is migration? Migration = Erosion Transport Deposition Re-erosion • Not an operational issue in today’s tokamaks, but certainly will be in ITER and beyond ……
Migration will be important • Co-deposition • High erosion rates and long term migration of carbon yield high levels of Tritium retention • ITER: ~50 g T per pulse • 0.01-0.2 g per pulse now • ITER operation suspended once 350 g T accumulated • Could be fewer than ~100 pulsesNo proven T clean-up technology • Material mixing, properties • Formation of compounds and alloys through the interaction of pure materials • Change of material properties • Be on W forms BeW alloys already at ~800°C • Surface melting point could be ~2000°C lower than for pure W
t = 3.0 s • t = 12.0 s Limited Diverted Where do erosion and migration occur? • JET #62218: plasma visible light emission At specific structures to protect the vacuum vessel walls or isolate the plasma-surface interaction
Some terminology Poloidal cross-section • Scrape-off layer (SOL) • Cool plasma on open field lines • SOL width ~1 cm ( B) • Length usually 10’s m (|| B) Core plasma • Divertor • Plasma guided along field lines to targets remote from core plasma: low T and high n Separatrix Private flux region Inner Outer • ITER will be a divertor tokamak Divertor targets
Materials in today’s tokamaks • The majority of today’s medium to large size tokamaks favour Carbon extensive operational experience • No melting / low core radiation / high edge radiation • But T-retention problem and high erosion rates of low Z mean that high Z may be the only long term solution • Living with W: see Kallenbach, I3.004, Wed.
Migration = Erosion Transport Deposition Re-erosion
Principal erosion mechanisms • Sputtering • Ions and neutrals • Physical and chemical (for carbon) • Macroscopic - transients • Melt layer losses • Evaporation, sublimation • Not generally observed in present experiments – currently the main reason for Carbon being used in the ITER divertor • Arcing, Dust (see Krasheninnikov et al, P4.019, Thurs.)
Eckstein et al. • Roth et al., NF 44 (2004) L21 • ITER divertor flux • D impact Physical and chemical sputtering • Physical • Chemical (carbon) • No threshold • Dependent on bombarding energy, flux and surface temperature • More optimistic prediction for ITER • Energy threshold higher for higher Z substrate • Much higher yields for high Z projectiles
ELMs: an example of transient erosion • Da • t = 19.05 s, ELM-free • t = 19.06 s, Type I ELM • JET #62218 • H-mode Edge MHD instabilities Periodic bursts of particles and energy into the SOL. Type I ELMing H-mode is baseline ITER scenario • Time (s) • For more on the physics of ELMs, See Huysmans, I4.002 Thurs.
ELMs can ablate Carbon on JET Radiated Power 1.0 MJ ELM 19.79 s ELM-free 19.73 s • 1 MJ ELM ~0.2 MJm-2 on the divertor target • Peak Tsurf ~ 2500ºC • Range of energies expected per Type I ELM in ITER ~ 0.6 3.5 MJm-2 • Loarte et al, Phys. Plasmas 11 (2004) 2668
ELM ablation limits ITER divertor lifetime Inter-ELM power: 5 MWm-2 Target thickness:CFC: 20 mmW: 10 mm No redeposition of ablated material No W melt layer loss ITER min. requirement W CFC • Minimum ITER ELM size • Federici et al, PPCF 45 (2003) 1523 Acceptable lifetime before target change required: • 3000 full power shots ~1 x 106 ELMs • Both low and high Z target materials marginal on present scalings • Significant effort in the community towards ELM mitigation
Migration = Erosion Transport Deposition Re-erosion
Transport creates & moves impurities • Gas puff • CX event • Ionisation Neutrals: • From divertor plasma leakage, gas puffs, bypass leaks low energy CX fluxes wall sputtering • Lower fluxes of energetic D0 from deeper in the core plasma • Escape via divertor plasma • Bypass leaks • EDGE2D/NIMBUS Ions: Cross-field transport – high ion fluxes can extend into far SOL recycled neutrals direct impurity releaseELMs ….. Eroded Impurity ions “leak” out of the divertor (T forces) SOL and divertor ion fluid flows– can entrain impurities
Bj ● Experimentally, strong SOL flows • D-flows: parallel Mach Number, M = v||/cs. POSITIVE towards inner target M M JET (Tore-Supra) C-Mod JT-60U (TCV) M N. Asakura, NF 44 (2004) 503 B. LaBombard, NF 44 (2004) 1047 S. K. Erents, PPCF 46 (2004) 1757 JT-60U M M JT-60U Distance to separatrix (mm) Distance to separatrix (mm) • See LaBombard, I3.007 Wed., Bonnin, P2.110, today
Using tracers to study the transport • 13CH4 markers are being increasingly used to get a handle on migration • gas puff just before vent and tile retrieval – pioneered on TEXTOR • 0.2g 13C, L-mode • 2.8g 13C, ohmic • 0.2g 13C, H-mode JET DIII-D AUG • 0.0025g 13C H-mode • 9.3g 13C H-mode
Top injection: C13 inner target • Wampler et al, JNM 337-339 (2005) 134 • Likonen et al, Fus. Eng. Design 66-68 (2003) 219 JET Start End DIII-D • Simple conditions: ohmic, L-mode, no ELMs • DIII-D: toroidally symmetric injection, JET: toroidally localised • Data and modelling demonstrate fast flow to inner divertor • Situation more complex in H-mode and other injection points • For more on JET C13 expts. see Rubel, P2.004, today
Migration = Erosion Transport Deposition Re-erosion
Deposition sensitive to local conditions DIII-D • Outer divertor usually hotter favours C erosion (phys. + chem.) • Inner divertor usually colder favours C deposition (chem. only) • C transport by SOL flows • Similar picture on most other carbon machines • Observations consistent with a contribution to the carbon source from outside the divertor Detached • Groth et al., P4.015, Thurs. • Whyte et al., NF 41 (2001) 1243, NF 39 (1999) 1025
1.2 1.0 Quartz Micro-Balance (QMB) 0.8 0.6 0.4 0.2 0.0 57084 Strike point 57080 57082 57086 Shot number Re-erosion important for C-migration • Esser et al., JNM 337-339 (2005) 84 JET • L-mode C-deposition (nm/s) • ERO code • Reproduced by transport modelling • Large increase on baseplate requires enhanced C re-erosion • Chemical erosion • Migration to remote areas due to magnetic and divertor geometry • Kirschner et al, JNM 337-339 (2005) 17
Global migration accounting = Erosion Transport Deposition Re-erosion
Tore Supra A non-trivial task! • Spectroscopic methods in plasma, post-mortem surface analysis and just plain old scraping and sweeping up extremely rigorous balance achieved first on TEXTOR (Wienhold et al., JNM 313-316 (2003) 311) • Tore Supra balance: see Dufour et al, P5.002 Friday
JET migration accounting (I) • Use spectroscopic methods + modelling to compute C sources EDGE2D/NIMBUS DIVIMP/OSMSimulation of CIII emission intrinsic sources 1 ton/year Divertor C-source = 5-10 x Wall source • Strachan et al, NF 43 (2003) 922 Carbon recycles
450g C (CIII) ~400g C JET migration accounting (II) • Make balance for period 1999-2001 with MarkII GasBox divertor: 14 hours plasmain diverted phase (50400 s, 5748 shots) • Spectroscopy + Modelling • Post mortem surface analysis • Deposition all at inner target • Net erosion at main walls • No significant divertor erosion • 215 kg/year strong T co-deposition • (1 year = 3.2 x 107 secs) • Very similar result for AUG, but overall C-balance more complex • Mayer et al, JNM 337-339 (2005) 119 • Likonen et al, JNM 337-339 (2005) 60, Matthews et al., EPS 2003
W+ W0 Tungsten migration in AUG • 2002-2003 Campaign: ~1.4 hours in diverted phase (4680 s, 1205 shots) • Post mortem surface analysis: • Only ~12% of inboard W source deposited in divertor • ~ few % to upper divertor and other main chamber surfaces W-coated: (40% of total area) 1.3x1018s-1 • W erosion not balanced by non-local deposition – most is promptly redeposited simpler than C picture • Larger Larmor radius helps at higher mass • ~1.5 kg/year 0.5x1017s-1 1.1x1017s-1 • Krieger et al, JNM 337-339 (2005) 10
Material choices for the next step An ITER-like first wall at JET
Current materials choice for ITER • Be for the first wall • Low T-retention • Low Z • Good oxygen getter W • C for the targets • Low Z • Does not melt 350 MJ stored energy • W for the baffles • High threshold for CX neutral sputtering CFC • Fallback option • Be wall, all-W divertor • Castellations for stress relief co-deposition in gaps? • Driven by the need for operational flexibility
Be Option 1 Option 2 An ITER-like wall in JET • Option 1 or 2 to be chosen in 2006: Objectives • Demonstrate low T-retention • Study melt layer loss (walls and divertor) ELMs and disruptions • Study effect of Be on W erosion • Be and W migration • Demonstrate operation without C radiation • Refine control/mitigation techniques ELMs and disruptions • Demonstrate routine / safe operation of fully integrated ITER compatible scenarios at 3-5MA Power upgrade to 40-45 MW • Experiments from 2009 onwards
Conclusions • Erosion and migration: Complex materials and physics • Not an operational issue now • But will be in ITER and beyond • Optimisation of core plasma performance and wall lifetime cannot be decoupled • Refine predictive capability • Still significant uncertainties ……. Full wall materials tests in current machines
ELMs might also erode the main walls • Main chamber thermography on AUG • A. Herrmann, AUG • Type I ELMs: ~25% of stored energy drop deposited on non-divertor components • ELM ion energies measured at JET walls agree with recent theory • Suggests:Eion > 1 keV on ITER erosion problem, even for high Z wall • Herrmann et al, P1.006 Mon.
ErxB, pxB EqxB Ballooning Pfirsch-Schlüter Divertor sink Can SOL ion flows transport material? • Yes, but picture is complex – theory and experiment not yet reconciled • Poloidal Bj • Parallel • Simplified – shown in the poloidal plane only
Carbon balance: TEXTOR, Tore Supra • Carbon Sources (g/h) von Seggern et al, Mayer et al., Phys. Scripta T111 (2004) Wienhold et al, von. Seggern et al., JNM 313-316 (2003)Brosset et al., JNM 337-339 (2005) 311, E. Tsitrone et al., IAEA 2004 TEXTOR TS Toroidal limiters: 22 7 • Carbon Sinks (g/h) Toroidal limiters: 10 1 “Obstacles”: 6 0.5 Low sticking – also AUG Bumper: 1 ? Neutralisers: 1 1-2 • Very good balance considering the scope for error • TEXTOR deposition extrapolates to~220 kg/year of plasma • Tore-Supra balance still preliminary Pump ducts: 0.02 ? Pumped out: 1-2 0.2-2 Total: 19-20 2.7-5.5 • Dufour et al, P5.002 Friday
Similar observations at JET • Net inner divertor deposition and little net erosion in outer divertor implies net wall source • Macroscopic flakes in regions not generally visible to plasma migration to remote areas high levels of T-retention Flakes • Coad et al., JNM 313-316 (2003) 419
20gBe (BeII) 450gC (CIII) 22g Be ~400g C JET migration accounting (II) • Make balance for period 1999-2001 with MarkII GasBox divertor: 16 hours plasma • Spectroscopy + Modelling • Post mortem surface analysis • Deposition all at inner divertor • Surface layers are Be rich Cchemically eroded and migrates, Be stays put • 215 kg/year strong T co-deposition • Very similar result for AUG, but overall C-balance more complex • Mayer et al, JNM 337-339 (2005) 119 • Likonen et al, JNM 337-339 (2005) 60, Matthews et al., EPS 2003