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EXPERIMENTS WITH LARGE GAMMA DETECTOR ARRAYS Lecture IV

EXPERIMENTS WITH LARGE GAMMA DETECTOR ARRAYS Lecture IV. Ranjan Bhowmik Inter University Accelerator Centre New Delhi -110067. ASSIGNMENT OF SPIN & PARITY. General Properties of Electromagnetic Radiation.

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EXPERIMENTS WITH LARGE GAMMA DETECTOR ARRAYS Lecture IV

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  1. EXPERIMENTS WITH LARGE GAMMA DETECTOR ARRAYSLecture IV Ranjan Bhowmik Inter University Accelerator Centre New Delhi -110067

  2. ASSIGNMENT OF SPIN & PARITY Lecture IV SERC-6 School March 13-April 2,2006

  3. General Properties of Electromagnetic Radiation • Individual nuclear states have unique spin and parity. For decay from (Ei Ji Mi pi ) to (Ef Jf Mf pf), the electromagnetic radiation must satisfy the following relations: • Energy Eg = Ei - Ef • Multipolarity|Ji - Jf| L  (Ji + Jf) • M-state M = Mi - Mf • Parity p = pipf For time varying field, the vector potential A should satisfy the vector Helmholtz equation : The scalar Helmholtz equation has the following solution with states of good angular momentum L and parity (-1)L Lecture IV SERC-6 School March 13-April 2,2006

  4. ELECTRIC & MAGNETIC TRANSITIONS • The corresponding Vector solutions are : Parity (-1)L+1 Parity (-1)L At large distances (kr » 1), Electric and magnetic fields complimentary : E(r ; E) = H(r ; M) H(r ; E) = -E(r ; M) At short distances (kr « 1 ) |E(r ; E)| >> |H(r ; E)| |H(r ; M)| >> |E(r ; M)| This justifies the names 'Electric' and 'Magnetic' for the two types of fields. Electric field interacts with charges  Electric multipole excitation Magnetic field interacts with currents (magnets)  Magnetic multipole excitation Lecture IV SERC-6 School March 13-April 2,2006

  5. ELECTRIC DIPOLE RADIATION • The classical radiation field from an oscillating dipole is given by • P ~ E  H ~ sin2q  r2 • which is maximum in a plane  to dipole direction [ zero at 0] • The electric field is in the plane containing the dipole. • Quantum mechanically, this correspond to a dipole field with L=1 M=0 with linear polarization along q P • For an axially symmetric oscillating quadrupole field (Q20) the radiation pattern P ~ E  H ~ sin2qcos2q  r2 [ zero at 0 & 90] • Quadrupole field with L=2 M=0 with linear polarization along q Lecture IV SERC-6 School March 13-April 2,2006

  6. ANGULAR DISTRIBUTION OF MULTIPOLE RADIATION • Angular distribution Z(W) =| A(r,q,f) |2 is a function of q only • For magnetic radiation, role of E & H are interchanged • Similar angular distribution for electric and magnetic multipoles • would differ in plane of polarization • Adding all the M components incoherently would result in isotropic unpolarized radiation • Electric dipoleradiation at 90 • Polarization M = 0 || to axisM = 1  to axis • Electric Quadrupole radiation at 90 Polarization M = 1 || to axis M =2  to axis Lecture IV SERC-6 School March 13-April 2,2006

  7. ELECTROMAGNETIC TRANSITION PROBABILITY The transition probability for the nucleus decaying from a state |JiMi > to state |JfMf > by an interaction R is given by • Since we are not interested in the orientation of either the initial or the final nucleus, we sum over all Mf and average over all Mi . Angular distribution of the photon would involve contributions from different allowed values of L & M. Since kR « 1, the transition probabilityTfi decrease rapidly with L and the lowest allowed L is important. Lecture IV SERC-6 School March 13-April 2,2006

  8. MULTIPOLARITY OF TRANSITION • For a change in angular momentum DL = |Ji - Jf| the dominant multipolarities are : M1 & E2often have comparable strength Lecture IV SERC-6 School March 13-April 2,2006

  9. RADIATION FROM ORIENTED NUCLEI • Random orientation of nuclei : radiation is isotropic as all Mi substates are to be added incoherently:radioactive decay • Nuclei oriented perpendicular to z-axis:fusion • Populates large spins with Mi ~ 0 by heavy ion fusion • Mi 0 nuclei decaying predominantly to Mf  0 For L=1 M = 0 • Emitted radiation maximum at q ~ 90 • Polarization || to z-axis for Electric transition For L=2 M = 0,  1 • Emitted radiation minimum at q ~ 90 • Polarization || to z-axis for Electric transition L=DJ for stretched transition • Nuclei oriented along z-axis : polarized nuclei M = LAngular distribution opposite; polarization reversed in sign Lecture IV SERC-6 School March 13-April 2,2006

  10. ALIGNMENT IN NUCLEAR REACTION • In fusion reaction between even-even nuclei, compound nucleus is populated with high spin at M=0 state. Successive particle emission would broaden the M-distribution. • Since the g-decay along the cascade is mostly stretched in nature (DJ =L) the M-distribution of the decaying state Ji would be centered around M=0 • If the spin distribution is symmetric i.e. P(-M) = P(M) NUCLEAR ALIGNMENT • Asymmetric spin distribution P(M) > P(-M) leads to NUCLEAR POLARIZATION Gaussian parameterization for oriented nuclei: P(Mi) ~ exp(-Mi2/s2)/Si exp(-Mi2/s2) with s/Ji ~ 0.3 Lecture IV SERC-6 School March 13-April 2,2006

  11. ANGULAR DISTRIBUTION IN FUSION • Angular distribution of g-transitions can be measured by moving the detector to a different q and normalising the counting rate w.r.t. a fixed detector • Shows pronounced anisotropy : • W(q) = 1 +a2P2(cosq) +a4P4(cosq) • Symmetric about 90 • W(q) = W(p - q) • Only even orders allowed with Nmax  2L • 'Beam in' & 'Beam out' directions equivalent Nucl. Phys. A95(1967)357 Lecture IV SERC-6 School March 13-April 2,2006

  12. Theoretical angular Distribution • The theoretical angular distribution from a state Ji to a state Jf by multipole radiation of order L, L' can be written as : where rK Statistical Tensor describing initial state population. Only even K allowed for symmetric M distribution Depends on the population width s Normalize to transitions with known multipolarity AK Geometrical factor depending on 3j, 6j, 9j symbols Sensitive to L-change in the high spin limit AK(JiLL'Jf) ~ AK(DJ,L) Lecture IV SERC-6 School March 13-April 2,2006

  13. ANUGULAR DISTRIBUTION FOR PURE MULTIPOLES • Angular distribution coeffs for pure multipoles in high spin limit for ideal initial M-distribution P(M) =1 for M=0 or  ½ Lecture IV SERC-6 School March 13-April 2,2006

  14. SYSTEMATICS OF L=2 TRANSITIONS • Angular distributions for DJ =2 very similar with a minimum at 90 • For most transitions • a2 = +0.30  0.09 • a4 = -0.09  0.05 • 20 transitions show large deviation due to external perturbation • Large anisotropy consistent with a narrow M-distribution s ~ 0.3 J PRL16(1966)1205 Lecture IV SERC-6 School March 13-April 2,2006

  15. SYSTEMATICS OF DIPOLE TRANSITIONS • Dipole transitions have a maximum at 90 • a2 -ve -a2 ~ 0.4 - 0.6 • If there is no change in parity, M1 can be mixed with E2 transitions • Angular distribution sensitive to the mixing ratio d • As the transitions are weak L=1 mostly seen in coincidence measurements E2 PRL16(1966)1205 M1,E2 Lecture IV SERC-6 School March 13-April 2,2006

  16. MIXING RATIO d • If for transition between states Ji Jf two multipolarities L, L' are allowed, d is the ratio of the reduced nuclear matrix elements • d a real number -     • Sign of d depends on the relative phase of the nuclear matrix elements • Angular distribution To extract d from measured W(q), rK must be estimated from a model of P(M) or extracted from pure E2 angular distribution Lecture IV SERC-6 School March 13-April 2,2006

  17. DETERMINATION OF MIXING RATIO d • Angular distribution of g-rays sensitive to DJ and mixing ratio • Solid curve : pure L=2 • Dotted curve : pure L=1 • Dashed & dot-dashed curve: • mixed transition d = -1 & +1 • Large interference effects for DJ =1 • Knowledge of both a2 & a4 important to identify the spin change DJ Lecture IV SERC-6 School March 13-April 2,2006

  18. ANGULAR CORRELATION • Weak transitions in a g-cascade can only be identified in g-g coincidence measurements • Angular correlation W(q1, q2, f) can be calculated theoretically if M-state population is known with sum over all variables K, K1, K2, q1, q2 For decay from symmetric M-distribution all K are even Lecture IV SERC-6 School March 13-April 2,2006

  19. ANGULAR CORRELATION • As a special case, we consider radioactive decay of a cascade of g-transitions. Because of the random orientation of the 4+ state populated by b-decay, all rK zero. By summing over all other indices the angular correlation is obtained as : where AK(1), AK(2) are the coefficients characterising the two transitions and q is the angle between the detectors. Lecture IV SERC-6 School March 13-April 2,2006

  20. ANGLAR CORRELATION : SYMMETRY PROPERTIES • Symmetric M distribution, 'beam in' & 'beam out' equivalent • W(q1,q2, f) = W( p - q1, p - q2, f) • Additional symmetries involving f p - f and f p +f • NIMA313(1992)421 • Integration over out-of-plane angle f product of angular distributions NPA563(1993)301 • Integration over angle of one detector Integration over all detectors gives the angular distribution Angular distribution from angular correlations using large array Lecture IV SERC-6 School March 13-April 2,2006

  21. Similarity between angular distribution & angular correlation Lecture IV SERC-6 School March 13-April 2,2006

  22. Anisotropy in angular distribution PRC53(1996)2682 • 'Gated angular distribution' extracted from the angular correlation W(q1,q2) by summing over all q2 • Anisotropy defined as E2 E1 M1/E2 E2/M1 where qA ~ 0 or 180 qB ~ 90 • Sensitive to DJ & d • Gating with unknown L possible Mixing Angle Three possible solutions !! need linear polarization data Lecture IV SERC-6 School March 13-April 2,2006

  23. Directional Correlation from Oriented Nuclei • Useful information about DJ can be obtained by measuringcoincidences between two detectors, one near 90 and the other near 0 with respect to beam direction • If the detectors are sensitive to both radiations g1 & g2 we can distinguish between • (i) g1 in detector 1 • g2 in detector 2 • (ii) g2 in detector 1 • g1 in detector 2 DCO = W(g1,q1; g2,q2)/W(g1,q2; g2,q1) Lecture IV SERC-6 School March 13-April 2,2006

  24. DCO Ratio • Ignoring f dependence we get • DCO ratio ~ [W(g1;q1)*W(g2; q2)] / [W(g1; q2)*W(g2; q1)] • = [W(g1; q1)/ W(g1; q2)] * [W(g2; q2)/W(g2; q1)] • If both radiations g1 and g2 have the same multipolarity, they have similar angular distribution and DCO ratio =1 • If they have different multipolarity i.e. L=1 for g1 and L=2 for g2 both terms greater than 1 and DCO ~ 2 • Exchange of angles or exchange of gating multipolarity would invert the ratio • Generalization valid only for Stretched transitions ! • Some papers have inverted definition i.e. NIMA275(1989)333 Lecture IV SERC-6 School March 13-April 2,2006

  25. EXPERIMENTAL DCO RATIO • Gate on E2 transition • 607 keV transition E2 • 484, 506, 516, 568, 617 keV transitions dipole 93Tc E2 gate PRC47(1993)87 Lecture IV SERC-6 School March 13-April 2,2006

  26. DCO Ratio : advantages • Can be used for weak transitions • More sensitive to angular distribution i.e. W(q)2 • Ideal for small arrays with limited number of angle combinations • Not overly sensitive to choice of angles • 75 < q1 < 105 • q2 < 30 or q2 >150 • DCO similar for both M1 & E2 transitions if DJ =1 • Large interference effect for mixed transitions • DCO ambiguity for DJ=0, 1 gate on L=2 q1=90 f =0 Lecture IV SERC-6 School March 13-April 2,2006

  27. Sensitivity of DCO Ratio to mixing parameter EPJA17(2003)153 Two solutions, need polarization data !! Lecture IV SERC-6 School March 13-April 2,2006

  28. POLARIZATION MEASUREMENTS • Angular distribution for both E1 and M1 similar; maximum at 90 • Can be distinguished by polarization measurement • Stretched E1 transition has polarization vector in-plane • stretched M1 transition has polarization vector perpendicular to plane • Maximum polarization at q = 90 • Can be studied in • (i) singles • (ii) in coincidence with another detector (PDCO) • (iii) measuring polarization of both detectors (PPCO) RMP31(1959)711 NIM163(1979)377 NIMA362(1995)556 NIMA378(1996)516 NIMA430(1999)260 Lecture IV SERC-6 School March 13-April 2,2006

  29. POLARIZATION FORMALISM • Polarization in a nuclear reaction : • where J0 , J90 are the average intensities of the Electric vector in plane with the beam direction & perp. to the plane. • Angular distribution : • Polarization : • Maximum at 90 with a value • for pure E1, M1 or E2: • P = +1 (E1,E2) ; -1 (M1) Lecture IV SERC-6 School March 13-April 2,2006

  30. Measurement of Polarization • Compton Scattering is sensitive to the polarization direction • Vertically polarized photons would be preferentially scattered in the horizontal plane • Klein-Nishina formula • Maximum sensitivity at q ~ 90 Lecture IV SERC-6 School March 13-April 2,2006

  31. Detection of Compton-scattered radiation • Two Ge detectors : one as scatterer and other as detector of scattered radiation • Need large efficiency for coincident detection • Identified as Eg = E1 + E2 • Experimental Asymmetry a(Eg) corrects for any instrumental effect between horizontal & vertical plane Lecture IV SERC-6 School March 13-April 2,2006

  32. Different Designs of Polarimeter CLOVER GAMMASPHERE Lecture IV SERC-6 School March 13-April 2,2006

  33. CLOVER as a Polarimeter • Polarization sensitivity • Q = A/P where P is polarization of the incident radiation • Large polarization sensitivity • Q ~ 13% at 1 MeV • Large Compton detection efficiency ~ 40% at 1 MeV • Measurement in singles or in coincidence NIMA362(1995)556 Lecture IV SERC-6 School March 13-April 2,2006

  34. Measurement of Polarization Electric Magnetic Lecture IV SERC-6 School March 13-April 2,2006

  35. Polarization Measurement in 163Lu PRL86(2001)5866 NPA703(2002)3 Lecture IV SERC-6 School March 13-April 2,2006

  36. Polarization measurement in 163Lu Confirmation of the wobbling mode in 163Lu through combined angular distribution and linear polarization measurement Lecture IV SERC-6 School March 13-April 2,2006

  37. Polarization-Direction Correlation PDCO Polarization-Polarization Correlation PPCO • With the availability of a large array of Clover detectors, we can measure the polarization of one or both g-rays in coincidence. This results in additional information in the form of PDCO (where one polarization is measured) or PPCO where both polarizations are measured. Combined with DCO this provides a powerful tool for spin assignment. I 4+ 2+ NIMA430(1999)260 Lecture IV SERC-6 School March 13-April 2,2006

  38. Lecture IV SERC-6 School March 13-April 2,2006

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