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January 22, 2003 MARAMA Mane-VU Science Meeting

Combined Aerosol & Trajectory Tool (CATT) Development R. Husar, K. Hoijarvi, J. Colson, S. Falke Center for Air Pollution Impact and Trend Analysis (CAPITA) Washington University in St. Louis Project Officer: Serpil Kayin MARAMA. January 22, 2003 MARAMA Mane-VU Science Meeting.

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January 22, 2003 MARAMA Mane-VU Science Meeting

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  1. Combined Aerosol & Trajectory Tool (CATT)DevelopmentR. Husar, K. Hoijarvi, J. Colson, S. FalkeCenter for Air Pollution Impact and Trend Analysis (CAPITA)Washington University in St. LouisProject Officer: Serpil KayinMARAMA January 22, 2003 MARAMA Mane-VU Science Meeting

  2. Project Background • The source-receptor relationship of particulate matter can be estimated by a number of empirical observation-based techniques. Some techniques are based chemical fingerprinting others on meteorological transport techniques. • A particularly attractive source-attribution technique, Paired Aerosol / Trajectory Analysis developed by Poirot and Wishinski. It combines the chemical and transport techniques by: • Establishing the major aerosol types at a specific receptor location and time (PMF and UNMIX) • Estimating the geographic transport regions for each aerosol type (Residence Time Analysis)

  3. Secondary Coal Avg. Mass: 3.2 ug/m3 (42%) Species: S, OC, EC, Na Summer Maximum Biomass Smoke Avg. Mass: 2.4 ug/m3 (32%) Species: OC, EC, S, K Summer Maximum East Coast Residual Oil Avg. Mass: 0.38 ug/m3 (5%) Species: OC, EC, S, Si, Ni, V Winter Maximum Illustration of Paired Chemical and Trajectory Analysis, Lye Brook, NH Wishinski and Poirot (2002)Based on Positive Matrix Factorization, PMF results from B. Coutant and ATAD trajectories from K. Gebhart High Secondary Coal contribution (yellow-red) originates from Upper Ohio River region Low Secondary Coal values (green-blue) occur during transport from Quebec High Biomass Smoke is transported from the N-NW direction Low Biomass Smoke occurs during transport from Quebec and the Ohio RV Region High Residual Oil aerosol type is transported from the East Coast Megalopolis Low Residual Oil occurs during transport from Quebec Project Goal: Develop an interactive data query and analysis tool for the paired chemical/trajectory analysis

  4. Typical Source Profiles Prepared by Battelle and Sonoma Tech. Inc. Data Input: PMF/UNMIX Source Profiles and Residence Time Residence Time (calculated as “hours per 80 x 80 km grid cell”) at each 16 site and receptor day, were calculated by P. Wishinski, VT DEC The ResTime calculations are based on daily ATAD trajectories provided K. Gebhart, CIRA. Source attribution results (PMF and UNMIX) for 16 receptor sites between Illinois and New England using IMPROVE and CastNet data have been completed by a previous project. The results of the Battelle/Sonoma PMF and UNMIX modeling are source profile time series for each location

  5. Project Objectives • Implement a relational database that incorporates both the PMF/UNMIX results and gridded trajectory data. • Develop specific SQL filtering and aggregation queries for • aggregated trajectory data based on chemical specifications • aggregated chemical data based on geographic specifications • Develop a graphic interface for user input (query) and for data output as rendered images or as exportable numeric data. • Transfer the resulting database to a designated SQL server and provide instructions for the addition of chemical and trajectory data.

  6. PMF/UNMIX Data ATAD Residence Time Relational Database • PMF and UNMIX data transfer to SQL • The PMF and UNMIX results were provided to us as Excel spreadsheet. • The metadata for the PMF and UNMIX were obtained verbally from R. Poirot. • The spreadsheet data were reformatted and imported in the SQL server two tables (ChemFactTable and LocTable) • Residence Time data transfer to SQL • The residence time data were provided by P. Wishinski on CDROM including full metadata documentation • The data were imported into two SQL tables (ResTimeFactTable and LocTable) CAPITA SQL Database

  7. Database Structure The dTrajResTime and dSourceApptables share the site_code and date keys thereby allowing paired queries to the SQL database.

  8. SQL Queries SELECT Lat as lat, Lon as lon, Loc_Code as loc_code, SUM(ResTime) AS [VALUE] FROM dTrajResTime WHERE ([Date] IN (SELECT datetime FROM dSourceApp WHERE (Loc_Code = 'loc_code') sql_filter_clause)) GROUP BY GridCode, Lat, Lon, Loc_Code ORDER BY Lon ASC Settings that are unique to a specific query are designated by red text

  9. Browsing ATAD Trajectory and Residence Time • Residence time and ATAD trajectory data superimposed for June 1, 2000.

  10. Browsing Chemical Data Query/Retrieval/Rendering of chemical data from SQL server

  11. Gr. Smoky Mtn. 1998 Pattern of PMF Clusters c3, c5, c9 Paired Trajectory and Chemical Data

  12. Seasonal Residence Time Retrieval and Rendering Lye Brook, JJA Lye Brook, DJF Gr Smoky Mtn, JJA Gr Smoky Mt, DJF

  13. Paired Chemical ‘Source’/ResTime Data, LYE BROOK,PMF Source C6 Sulfate, Titanium ResTime for High C6 (BioSmoke?) Chemical Conditions ResTime for Low C6 (BioSmoke?) Chemical Conditions

  14. CATT data flow, processing, and rendering ‘View’ Processing Data Sources Multi-dimensional Data Cube Spatial Portrayal Spatial Overlay Aerosol Data Trajectory Time CATT Browser Spatial Slice CAPITA or transferred SQL RDB Wrapper Time Slice Time Portrayal Time Overlay Wrapper VIEWS Other Data (GIS, Met., …) Wrapper

  15. CATT Project Status Current effort to finalize queries and user interface ‘Public’ testing and user feedback is expected to being in April

  16. Secondary Coal Avg. Mass: 3.2 ug/m3 (42%) Species: S, OC, EC, Na Summer Maximum Biomass Smoke Avg. Mass: 2.4 ug/m3 (32%) Species: OC, EC, S, K Summer Maximum East Coast Residual Oil Avg. Mass: 0.38 ug/m3 (5%) Species: OC, EC, S, Si, Ni, V Winter Maximum Illustration of Paired Chemical and Trajectory Analysis, Lye Brook, NH Wishinski and Poirot (2002)Based on Positive Matrix Factorization, PMF results from B. Coutant and ATAD trajectories from K. Gebhart High Secondary Coal contribution (yellow-red) originates from Upper Ohio River region Low Secondary Coal values (green-blue) occur during transport from Quebec High Biomass Smoke is transported from the N-NW direction Low Biomass Smoke occurs during transport from Quebec and the Ohio RV Region High Residual Oil aerosol type is transported from the East Coast Megalopolis Low Residual Oil occurs during transport from Quebec Project Goal: Develop an interactive data query and analysis tool for the above paired chemical/trajectory analysis

  17. Project Deliverables • Implement a relational database that incorporates both the PMF/UNMIX results and for gridded trajectory data. • Develop specific SQL filtering and aggregation queries for • aggregated trajectory data based on chemical conditions • aggregated chemical data based on geographic conditions • Develop a graphic interface for user input (query) and for data output as renderd images or as exportable numeric data. • Transfer the resulting database to a designated SQL server and provide instructions for addition of chemical and trajectory data.

  18. Project Status/Summary • Relational Database of PMF/UNMIX and trajectory data: Complete • Develop specific SQL filtering and aggregation queries • Chemical filtering/aggregation: Developed, needs testing and feedback • Trajectory filtering/aggregation: Developed, needs testing and feedback • Paired Chemical/Trajectory data: Partially developed, needs user input, testing, feedback • Graphic interface for user input (query) and for data output: Partially developed, needs user input, testing, feedback • Transfer the resulting database to a designated SQL server: Not done Project Milestones Jan-June 2003 • Feb 1, 03: Complete initial queries, user interface and displays • Apr 1, 03: Finalize design/implementation of queries, user interface and displays • Apr-Jun 03: ‘Public’ testing and user feedback • July 03: Tool delivery

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