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Presented by: S. M. Hosseini Pooya (PhD) National Radiation Protection Department

Development of a diffusion chamber for passive discriminative measurements of radon/ thoron concentration in dwellings. F. Torabi Nabil , S. M. Hosseini Pooya , M. Taheri , M . Shamsaie Zafarghandi. Presented by: S. M. Hosseini Pooya (PhD) National Radiation Protection Department

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Presented by: S. M. Hosseini Pooya (PhD) National Radiation Protection Department

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  1. Development of a diffusion chamber for passive discriminative measurements of radon/thoron concentration in dwellings F. TorabiNabil, S. M. HosseiniPooya, M. Taheri,M. ShamsaieZafarghandi Presented by: S. M. HosseiniPooya (PhD) National Radiation Protection Department Iran Nuclear Regulatory Authority

  2. Introduction • Radon (222Rn) has the most contribution in annually natural exposure of the human via inhalation of the gas. • Thoron (220Rn) may have the same effects (even be more hazardous) due to the long lived of its daughters . • As well most of the radon detectors are also sensitive to the thoron and may be affected on accurate measurements by the presence of thoron in media. • Thus some of the researches are focused on the designing of discriminative systems for separated measurements of these isotopes. • Most of the suggested systems have complicated designs (in active methods) and etching conditions (in passive methods). • A home-made passive diffusion chamber which is based on SSNTD, has been used for many years for passive radon measurements in dwellings in Iran. • In this research first the operation and calibration method of the chamber have been described for both radon and thoron measurements. • Then the design is developed for separated measurements of radon/thoron, and the measurement characteristics of the detector are discussed in detail.

  3. Structure of home-made diffusion chamber: for Radon measurements

  4. 4 Electrochemical Etching (ECE) Voltage:800 V Frequency: 2 kHz Time: 3 hr Temp.:25 ° C H2O)45% + C2H5OH40% + KOH15%Etchant PEW:

  5. Calibration Method The volume of calibration chamber for Radon is 50 liters and for Thoron is 4 liters

  6. The calibration curve of the chamber for Radon The calibration curve of the chamber for Thoron S= 13.55 (Track.cm-2.Bq-1 .l .day-1) S= 0.83 (Track.cm-2.Bq-1 .l .day-1)

  7. Results of the chamber response in the 4th International Intercomparison of Passive Radon Detectors (by NIRS –Japan, 2011)

  8. Developed diffusion chambers for discriminative measurement of radon and thoron Double-filter diffusion chamber & 212Po detector Double-film diffusion chamber

  9. Developed diffusion chamber: Radon detector the outside detector: 212Po detector Double-filter diffusion chamber + 212Po detector Attenuator(Lexan 75µm) • It attenuates only the particles of 8.78 MeV of 212Po to the energies between 0.5 to 1MeV and absorbs all of the other particles of the daughters. Detector(Lexan 250µm) Detector holder

  10. attenuator • The thickness of 75±2 μm has been calculated by Trim Code • The thickness of 75±2μm is achievable by soaking of the 250μm Lexan films in the Aqueous solution of Ethylenediaminefor 4 hours at 25⃘C as : 75% C2H4(NH2)2+25% H2O

  11. Sensitivity of the diffusion chamber for radon measurements The MDL values of the diffusion chamber for radon measurements S= 8.95 (Track.cm-2.Bq-1 .l .day-1)

  12. Sensitivity of the outer Lexan film for 212Po measurements The MDL values of the outer Lexan film for 212Po measurements S=7.96 (Track.cm-2.Bq-1 .m3 .day-1)

  13. Calculation of Thoron Concentration • The outer Lexan film only can measure the concentration of 212Po CTn(Thoron concentration)can be calculated by: The average value of FTn(Equilibrium Factor) is 0.03 in dwellings, 0.913 is the Equilibrium Coefficient, 100/64 is the reverse value of branching ratio in decay chain of 212Po

  14. Cap & fiber glass filter Detector Detector holder Fiber glass filter Filter holder • The upper film detects Radon+ Thoron • The lower film detects only the Radon Detector Detector holder Double-film diffusion chamber

  15. Sensitivity of the diffusion chamber for radon measurements The MDL values of the diffusion chamber for radon measurements S(upper film)=2.06 S(lower film)=1.60

  16. Sensitivity of the diffusion chamber for Thoron measurements The MDL values of the diffusion chamber for Thoron measurements S=0.056(Track.cm-2.Bq-1 .l.day-1)

  17. Conclusion • A home-made passive diffusion chamber which is based on Lexan SSNTD, has been developed for simultaneous measurements of radon/thoron in dwellings. • The sensitivity of the chamber shows that it is appropriate for seasonal measurements of radon in an extended range of concentrations. • The sensitivity of the double-film chamber shows that it is appropriate for seasonal measurements of thoron in areas with high thoron concentrations, while the double-filter method is appropriate for that of low concentration . • The advantages of the method are including its small size, light weight and simple etching process.

  18. Thank you!

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