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Modeling of plasma/lithium-surface interactions in NSTX: status and key issues. J.N. Brooks, A. Hassanein, T. Sizyuk, J.P. Allain Purdue University 2 nd International Symposium on Lithium Applications for Fusion Devices, PPPL, April 27-29, 2011. Why analyze NSTX plasma/lithium interactions?.
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Modeling of plasma/lithium-surface interactions in NSTX: status and key issues J.N. Brooks, A. Hassanein, T. Sizyuk, J.P. Allain Purdue University 2nd International Symposium on Lithium Applications for Fusion Devices, PPPL, April 27-29, 2011
Why analyze NSTX plasma/lithium interactions? • Lithium has been used extensively in NSTX*--will likely continue. Modeling can help explain device performance. • Flowing liquid lithium is a promising candidate for future devices (Fusion Nuclear Science Facility, DEMO, etc.). Code validation & model improvement is possible, using NSTX data. Concerns for NSTX analysis: Much more difficult to model than future devices --- Transient conditions: ~1 second pulse --- Small device–edge/boundary effects dominate --- Lithium is not a flowing liquid (i.e., is static liquid or solid) --- Other materials present (C, Mo, etc.) --- Non-standard boundary conditions *H.W. Kugel, “NSTX Plasma Response to Lithium Coated Divertor”, PSI-19 (2010), J. Nuc. Mat. to be published. *C.H. Skinner et al., “Deuterium Retention in NSTX with lithium Conditioning”, ibid,. to be published.
Lithium modeling issues Lithium is the 2nd most complex surface material we have modeled (carbon is first due to chemical sputtering): • D trapping/pumping—highly dependent on surface content/structure • High vapor pressure • Temperature dependent sputtering & evaporation • Material-mixing issues: e.g. Li intercalation in carbon • Liquid vs. solid issues • Most (~2/3) sputtering is Li+ ions • Li+ ion redeposition in sheath and re-emission at surface
Past & Current Work-Lithium/NSTX Modeling • Liquid Lithium Divertor (LLD) plasma/surface interaction analysis [J.N. Brooks, J.P. Allain, T.D. Rognlien, R. Maingi., J. Nuc. Mat. 337-339(2005)1053] [J.P. Allain, J.N. Brooks, Nuclear Fusion 51(2011)023002] • static liquid lithium response, low-D recycle plasma • Lithium Inner Divertor (HIBD) • static (pure) liquid Li or solid Li surface, high D-recycle plasma • Mixed material analysis: Li + C on Mo inner divertor, high-D-recycle plasma surface evolution: composition and sputtering Li, C detailed analysis; e.g., sputtering of thin Li coatings on graphite
REDEP/WBC LLD Analysis TRIM-SP computed total Li sputter yields (ion+atom)
Interesting physics for sputtered lithium transport in the NSTX low-recycle plasma regime: • Large sputtered atom ionization mean free path, order of 10 cm • Large Li+1 gyroradius ( ~5 mm), due to low B field (0.5T) • Low collisionality of Li ions with plasma; due to high Te, low Ne • Kinetic, sub-gyro orbit analysis required (i.e. WBC code)
WBC Simulation of LLD sputtered lithium transport: 50 trajectories shown; 2-D 3-D UEDGE/NSTX GRID • Long mean free paths seen for ionization; subsequent long, complex, ion transport
NSTX Liquid Lithium Divertor Analysis-results Results are encouraging: --Moderate lithium sputtering; no runaway --Acceptable Li contamination: ~7% SOL, ~1% Core --Carbon (2%) flux to LLD appears acceptable --LLD could apparently handle higher heat flux
NSTX is replacing Row 1 Horizontal Inboard Divertor (HIBD) carbon tiles with molybdenum —To reduce carbon sputtering & core plasma carbon content. • We are analyzing Mo, C, Li HIBD (“inner divertor”) sputtering erosion and plasma contamination, with high-recycle plasma. REDEP/WBC NSTX Inner Divertor Analysis; with high-recycle plasma[with H. Kugel, R. Maingi, C. Skinner, et al.]
NSTX Inner Divertor High-Recycling Plasma Solution (J. Canik SOLPS code) R~1 Peak plasma values at divertor Ne ~ 1x1020 m-3 Te ~ 60 eV strike point
Plasma Sheath • Sheath affects transport of sputtered and evaporated Li, and other materials • NSTX has non-standard tokamak boundary conditions—can affect sheath • NSTX sheath analyzed with BPHI-3D code (w/o full turbulence model)
WBC NSTX Lithium Divertor analysis: transport summary for two plasma cases (100,000 histories/simulation) a Values from [J.P. Allain, J.N. Brooks, Nuclear Fusion 51(2011)023002] b 300 C surface assumed for D and Li on Li sputter yields c normal-to-surface; for sputtered Li atoms ionized in divertor region. d average for redeposited Li ions on respective divertor e includes sputtered atoms, and sheath-reflected sputtered ions re-emitted as atoms from surface. • Major differences, but acceptable lithium erosion/redeposition in both cases
WBC analysis: comparison of three surface materials NSTX inner divertor, high-recycle regime a with 1% C+3 and 1% Li+2 plasma impingement b normal-to-surface; for sputtered atoms ionized in divertor region. c numerical bound • C and Li net sputter erosion is about 5-10 times higher than Mo erosion • No material highly contaminates core plasma
Dynamic evolution of mixed materials bombarded with multiple ion beams: ITMC-DYN Computer Simulation Package ITMC-DYN Integrated Models • A. Hassanein, “Surface effects on sputtered atoms and their angular and energy dependence”, Fusion Technology 8 (1985) 1735. • T. Sizyuk and A. Hassanein, "Dynamic analysis and evolution of mixed materials bombarded with multiple ions beams", J. Nucl. Materials, 40( 2010)60 • T. Sizyuk and A. Hassanein “Dynamic analysis of mixed ion beams/materials effects on the performance of ITER-like devices“, to be publishedJ. Nucl. Mat. (2010)
ITMC-DYN analysis: time dependent sputtering of NSTX Mo inner divertor (at strike point); with D, 1% C, 1% Li impingement • Substantial carbon and lithium sputtering occurs by end-of-shot
ITMC-DYM Analysis: Spatial distribution of the deposited C and Li impurities in Mo substrate; NSTX Mo inner divertor (at strike point) • C and Li surface contamination extend to ~10 nm • C and Li concentrations peak at ~ 5 nm depth and about equal the Mo concentration
Conclusions-NSTX Lithium plasma/surface interactions • Analysis of lithium erosion/transport in NSTX is important, but highly complex. (Results uncertain due to complexity of lithium/NSTX modeling, and general issues in plasma predictive modeling.) Key focus is on mixed-material modeling. • The static liquid lithium divertor (LLD) with high-power, D-trapping plasma shots, is predicted to work well—from the (sputtering & evaporation) erosion standpoint. • A lithium surface—solid or liquid, for low or high D recycle plasma—has high erosion but low core plasma contamination potential (~0.1-1%). • A Mo surface may be substantially changed, in 1 second, by C and Li impingement. Mo core plasma contamination by sputtering appears low (<0.01%), in any event. (Not clear if Mo substantially reduces NSTX core plasma carbon content). • Continuing work: Other plasma solutions (e.g., inner Mo with outer low-recycle LLD), self-consistent material-mixing/evolution, data-calibrated model refinements. {Supercomputing needed for more complete plasma/material interaction analysis.}