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Superheavy nuclei: relativistic mean field outlook

Superheavy nuclei: relativistic mean field outlook. Anatoli Afanasjev. University of Notre Dame. Motivation 2. Reliability of RMF parametrizations 3. Is that possible to find some common ingredient in the predictions

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Superheavy nuclei: relativistic mean field outlook

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  1. Superheavy nuclei: relativistic mean field outlook Anatoli Afanasjev University of Notre Dame • Motivation • 2. Reliability of RMF parametrizations • 3. Is that possible to find some common ingredient in the predictions • of magic gaps in superheavy spherical nuclei?  Central depression • in the density and its impact on shell structure. • 4. Pairing in superheavy nuclei. • 5. Conclusions Disclaimer: few results with Gogny and Skyrme forces used in the present presentation are from J.-F. Berger et, NP A685 (2001) 1c and M. Bender et, PRC 60 (1999) 034304 In collaboration with Stefan Frauendorf

  2. Nucleonic densities Magic gaps in spherical superheavy nuclei Self-consistency Self-consistent theories give the largest variations in the predictions of magic gaps at Z=120, 126 and 172, 184 Single- particle spectra Potentials: nucleonic, spin-orbit 1. A pair of the RMF sets which indicate Z=114 and N=184 gaps are eliminated as candidates by performing the analysis of quasiparticle spectra in deformed nuclei in actinide region, A.V.Afanasjev et, PRC 67 (2003) 024303 protons neutrons Self- consistency 2. Skyrme SkI4 also predicts Z=114 (K. Rutz et al, PRC 56 (1997) 238) but it reproduces spin-orbit splitting very badly (M. Bender et, PRC 60 (1999) 034304) Circles are broken in the macroscopic- microscopic method which consistently predicts Z=114, N=184

  3. Reliability of parametrizations # of parametrizations: Skyrme > 80 RMF > 20 “All animals [theories, parametrizations] are equal, but some animals [theories, parametrizations] are more equal than others” George Orwell, ‘Animal farm’’ Goal: To find the RMF parametrizations best suited for the description of superheavy nuclei Method: perform detailed analysis of the spectroscopic data in the A~250 deformed mass region in the framework of cranked relativistic Hartree-Bogoliubov (CRHB) theory see A.V.Afanasjev et al, PRC 67 (2003) 024309 for results

  4. CRHB+LN results sometimes called as “2-nucleon gap” An analysis of experimental data only in terms of these quantities can be misleading Example of NLSH: indicates Z=100 gap but between wrong s-p states

  5. For each configuration (blocked solution) the binding energy Ei is calculated fully self- consistently (including also time-odd mean fields)

  6. RMF analysis of single-particle energies in spherical Z=120, N=172 nucleus corrected by the empirical shifts obtained in the detailed study of quasiparticle spectra in odd-mass nuclei of the deformed A~250 mass region (PRC 67 (2003) 024309) Self-consistent solution Pseudospin doublets 2g7/2-3d5/2 172 172 1i11/2-2g9/2 1h9/2-2f7/2

  7. Accuracy of the description of single-particle energies Best sets (NL1,NL3,NL-Z2) ---- for most subshells better than 0.5 MeV for a few subshells the discrepancies reach 0.7-1 MeV Worst sets (NLSH, NLRA1) --- much higher errors in the energies of single-particle states (the only sets which predict Z=114 as shell gap)  should be excluded Important: no-single particle information is used in the fit of the RMF forces Additional constraint by the study single-particle states in nuclei with N~162 and/or Z~108 Single-particle states are observed

  8. Macroscopic + microscopic approach predicts Z=114 and N=184, but basic assumptions (see below) are VIOLATED. pairing liquid drop quantum (shell) correction The radial density dependence used in liquid drop model FLAT DENSITY distribution in the central part of nucleus Woods-Saxon potential R0=r0A1/3 r0~1.2 fm a ~ 0.5 fm V0~50 MeV

  9. Lesson from quantum mechanics: spherical harmonic oscillator A B A: the radial wave function B: effective radial potential, i.e. with the centrifugal term added.

  10. Densities of superheavy nuclei: spherical RMF calculations with the NL3 force x

  11. The clustering of single-particle states into the groups of high- and low-j subshells is at the origin of the central depression in the nuclear density distribution in spherical superheavy nuclei.

  12. A.V.Afanasjev and S.Frauendorf, PRC 71, 024308 (2005) ‘g-s’ – ground state configuration ‘exc-s’ – excited state configuration Occupied state Unoccupied state p = + p = - 3p1/2 particle-hole excitation leading to flatter neutron and proton density distribution 126 3d5/2 Self-consistency effects related to density redistribution define the shell structure: Z=114 shell gap can be excluded Spherical RMF calculations with NL3 forces

  13. Impact of particle-hole excitations on the densities and potentials (nucleonic, spin-orbit) densities densities General conclusion (tested on large # of particle-hole excitations in different nuclei): potentials • Large density depression • in the central part of nucleus: • shell gaps at Z=120, • N=172 2. Flat density distribution in the central part of nucleus: Z=126 appears, N=184 becomes larger and Z=120 (N=172) shrink

  14. Skyrme SkP [m*/m=1] double shell closure at Z=126, N=184 (SkM*, ???? Large effective mass m*/m~0.8-1.0 Skyrme SkI3 [m*/m=0.57] gaps at Z=120, N=184 no double shell closure, SLy6 Which role effective mass plays??? Gogny D1S Z=120, N=172(?) Z=126, N=184 Low effective mass m*/m ~ 0.65 RMF double shell closure at Z=120,N=172

  15. Why macroscopic+microscopic • models are working so well • in known superheavy nuclei??? • They are deformed • Deformation leads to more equal distribution of the states emerging from high- and low-j subshells (and, thus, removes the clustering of high-j subshells seen in spherical superheavy nuclei). • This leads to almost flat density distributionin the central part of nucleus. • Single-particle features are fitted to experimental data CRHB+LN results

  16. The importance of particle number projection (PNP) in spherical superheavy nuclei Most of other calculations were performed with no PNP Pairing collapse at “magic” gaps Approximate PNP by Lipkin-Nogami (LN): no pairing collapse Calc. with no PNP overestimate d2p (“2-proton shell gap”)

  17. Stability against fission RMF - low barriers, Skyrme HF – high barriers Experiment: fission barrier heights in heavy actinides (A~240) RMF: somewhat underestimates Skyrme HF – overestimates by few MeV From M.Bender et al, PRC (2003)

  18. Conclusions • The central depression in density distribution of spherical superheavy • nuclei plays an important role in the definition of their shell structure: • Large density depression • in the central part of nucleus favors • shell gaps at Z=120, N=172 2. Flat density distribution in the central part of nucleus favors Z=126 and N=184 Intermediate situations appear dependent on the quality of force with respect of single-particle degrees of freedom (position of j-subshells, spin-orbit splitting, pseudospin splitting) The check of quality of force with respect of deformed single-particle states is MUST BE 2. 3. Particle number projection is important for proper description of pairing properties of spherical superheavy nuclei and calculation of indicators of low-level density (d2n – “2-nucleon gaps”)

  19. A.V.Afanasjev et al, PRC 67 (2003) 024309 Discrepancy between theory and experiment   empirical shifts for the positions of spherical subshells

  20. The Sleep of Reason Produces Monsters. (Caprichos, no. 43, Goya)

  21. How magic are “magic” shell gaps? Calculated spherical Z=120 gap versus experimental deformed Z=100 gap Similar relation for neutron spherical N=172 and deformed N=152 gap It might be that the effect of spherical shell gaps in superheavy nuclei is only 30-40% more pronounced than the effect of deformed gaps in the A~250 region

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